STUDY OF HEAVY METALS IN BOTTOM SEDIMENTS OF THE EAST CHINA SEAS (Bohai, Huanghai and the East China Sea):A REVIEW OF CURRENT STATUS
-
摘要: 中国东部海域(渤海、黄海和东海)底质沉积物接受了巨量的重金属(As、Cd、Cu、Cr、Hg、Ni、Pb、Zn和V),从而使得底质环境质量可能面临严重的重金属污染。这些重金属来源复杂,其中既有自然源重金属又有不同人为来源。其中自然源可能主要包括长江流域、黄河流域的泥沙和中国西部沙漠的粉尘,人为来源可能主要包括煤炭和燃油消耗、钢铁冶炼和有色金属冶炼,其中煤炭消耗和有色金属冶炼可能是中国东部海域沉积物铅和汞的最主要的来源。这些重金属主要通过河流输入的方式进入到中国东部海域,尽管鉴定沉积物中重金属具体人为来源的方法较多,但在中国东部海域应用最为成功的是铅稳定同位素。尽管巨量的重金属输入到中国东部海域,但绝大部分海域底质沉积物质量良好,仅在锦州湾海域重金属含量严重超标。Abstract: A great amount of heavy metals is discharged from large and small rivers into the Eastern China Seas, which include the Bohai, Huanghai and the East China Sea in total, and eventually preserved in the bottom sediments, which makes the marine environment faced with the serious heavy metal pollution. These heavy metals come from various sources, which may be generally put into natural and anthropogenic groups. The natural sources mainly include the eroded soils from the Yangtze River Basin and the Yellow River Basin and the desert dust from West China. The anthropogenic sources mainly include the pollution caused by human activities dominated by combustion of fossil fuels and smelting of steel and non-ferrous metals. These heavy metal contaminants are mainly discharged into the Chinese Eastern Seas through rivers. Various methods have been adopted to identify the sources of heavy metals in marine sediments, and the stable isotope of Pb is believed the most successful indicator. Although huge amounts of heavy metals have been discharged into the Chinese Eastern Seas, the marine sediment offshore remain in good quality, except the Jinzhou Bay which is faced with the serious heavy metal pollution.
-
Keywords:
- East China Seas /
- heavy metals /
- sources /
- fluxes /
- environment quality
-
-
[1] Cheng H, Hu Y. Lead (Pb) isotopic fingerprinting and its applications in lead pollution studies in China:a review[J]. Environmental Pollution, 2010, 158(5):1134-1146.
[2] Nriagu J O. Global inventory of natural and anthropogenic emissions of trace metals to the atmosphere[J].Nature, 1979,279(5712):409-411.
[3] Thevenon F, Guédron S, Chiaradia M, et al. (Pre-) historic changes in natural and anthropogenic heavy metals deposition inferred from two contrasting Swiss Alpine lakes[J]. Quaternary Science Reviews, 2011, 30(1):224-233.
[4] Elbaz-Poulichet F, Dezileau L, Freydier R, et al. A 3500-year record of Hg and Pb contamination in a Mediterranean sedimentary archive (The Pierre Blanche Lagoon, France)[J]. Environmental Science & Technology, 2011, 45(20):8642-8647.
[5] Blaser P, Zimmermann S, Luster J, et al. Critical examination of trace element enrichments and depletions in soils:As, Cr, Cu, Ni, Pb, and Zn in Swiss forest soils[J]. Science of the Total Environment, 2000, 249(1):257-280.
[6] Barbante C, Schwikowski M, Döring T, et al. Historical record of European emissions of heavy metals to the atmosphere since the 1650s from Alpine snow/ice cores drilled near Monte Rosa[J]. Environmental Science & Technology, 2004, 38(15):4085-4090.
[7] Morelli G, Gasparson M, Fierro D, et al, Historical trends in trace metal and sediment accumulation in intertidal sediment of Moreton Bay, southeast Queensland, Australia. Chemical Geology,2012:300-301, 152-164.
[8] 蓝先洪. 中国主要河口沉积物的重金属地球化学研究[J]. 海洋地质动态,2004, 20(12):1-4. [LAN Xianhong. Heavy metal geochmistry of sediments in the marine[J]. Marine Geology Letters, 2004, 20(12):1-4.]
[9] Pan K, Wang W X. Trace metal contamination in estuarine and coastal environments in China[J]. Science of the Total Environment, 2012, 421:3-16.
[10] 国家海洋局. 中国海洋环境公告. 2011.[National Bureau of Oceanography of China, 2011. Bulletin of Marine Environmental Quality.] [11] Ip C C M, Li X D, Zhang G, et al. Over one hundred years of trace metal fluxes in the sediments of the Pearl River Estuary, South China[J]. Environmental Pollution, 2004, 132(1):157-172.
[12] Yuan C, Shi J, He B, et al. Speciation of heavy metals in marine sediments from the East China Sea by ICP-MS with sequential extraction[J]. Environment International, 2004, 30(6):769-783.
[13] Yu Y, Song J, Li X, et al. Fractionation, sources and budgets of potential harmful elements in surface sediments of the East China Sea[J]. Marine Pollution Bulletin, 2013, 68(1):157-167.
[14] Chen B, Fan D J, Li W R, et al. Enrichment of heavy metals in the inner shelf mud of the East China Sea and its indication to human activity[J]. Continental Shelf Research, 2014, 90:163-169.
[15] 刘明,张爱滨,范德江,等. 渤海中部底质沉积物重金属环境质量[J]. 中国环境科学,2012,32(02):279-290. [LIU Ming, ZHANG Aibin, FAN Dejiang, et al. Environmental quality of heavy metals in surface sediments in the central region of the Bohai Sea[J]. China Environmental Science, 2012,32(02):279-290.]
[16] Zhang J, Huang W W, Liu S M, et al. Transport of particulate heavy metals towards the China Sea:a preliminary study and comparison[J]. Marine Chemistry, 1992, 40(3):161-178.
[17] Zhang W G, Feng H, Chang J N, et al. Heavy metal contamination in surface sediments of Yangtze River intertidal zone:an assessment from different indexes[J]. Environmental Pollution, 2009, 157(5):1533-1543.
[18] Nriagu J, Becker C. Volcanic emissions of mercury to the atmosphere:global and regional inventories[J]. Science of the Total Environment, 2003, 304(1):3-12.
[19] 洪汉净,刘辉. 火山活动状态及其机理的初步探讨[J]. 地震地质,2007,29(03):502-512. [HONG Hanzheng, LIU Hui. Preliminary study on Active States of Volcao and their mechanisms[J]. Seismology and Geology, 2007,29(03):502-512.]
[20] 田卫堂,胡维银,李军,等. 我国水土流失现状和防治对策分析[J]. 水土保持研究,2008,15(04):204-209. [TIAN Weitang, HU Weiyin, LI Jun,et al. The Status of Soil and Water Loss and Analysis of Countermeasures in China[J]. Research of Soil and Water Conservation, 2008, 15(04):204-209.]
[21] 赵一阳. 中国海大陆架沉积物地球化学的若干模式[J]. 地质科学,1983,04:307-314.[ZHAO Yiyang. Some Geochemical pattern of shelf sediments of the China Seas[J]. Scientia Geologica Sinica, 1983 , 04:307-314.]
[22] 中华人民共和国水利部和中华人民共和国国家统计局. 中国第一次水利普查公告[R]. 2013.[Ministry of Water Resources of the People's Republic of China and The bureau of the People's Republic of China. Bulletin of first national census for water[R]. 2013.] [23] 王宏,石广玉,王标,等. 中国沙漠沙尘气溶胶对沙漠源区及北太平洋地区大气辐射加热的影响[J]. 大气科学,2007,31(03):515-526. [WANG Hong, SHI Guangyu, WANG Biao, et al. The Impacts of Dust Aerosol from Deserts of China on the Radiative Heating Rate over Desert Sources and the North Pacific Region[J]. Chinese Journal of Atmospheric Sciences, 2007,31(03):515-526.]
[24] 杨杰东,陈骏,饶文波,等. 中国沙漠的同位素分区特征[J].地球化学,2007,36(05):516-524. [YANG Jiedong, CHEN Jun, RAO Wenbo, et al. Isotopic partition characteristics of Chinese deserts[J].Geochimica, 2007, 36(05):516-524.]
[25] 闫涵,高会旺,姚小红,等. 沙尘传输路径上气溶胶浓度与干沉降通量的粒径分布特征[J]. 气候与环境研究,2012,17(02):205-214. [YAN Han, GAO Huiwang, YAO Xiaohong, et al. Size-dependent mass and dry deposition fluxes of atmopheric aerosols along dust transport routes[J]. Climatic and Environmental Research, 17(02):205-214.]
[26] Fang T H, Li J Y, Feng H M, et al. Distribution and contamination of trace metals in surface sediments of the East China Sea[J]. Marine Environmental Research, 2009, 68(4):178-187.
[27] 中华人民共和国水利部。2008年中国河流泥沙公告[M]..北京:中国水利水电出版社,2009.[Ministry of Water Resources of the People's Republic of China. Bulletin of first national census for water[M]. Beijing:China Waterpower Press, 2009.] [28] Zhang X Y, Arimoto R, An Z S. Dust emission from Chinese desert sources linked to variations in atmospheric circulation[J]. Journal of Geophysical Research:Atmospheres (1984-2012), 1997, 102(D23):28041-28047.
[29] 迟清华,鄢明才. 应用地球化学元素丰度数据手册[M]. 北京:地质出版社,2007.[CHI Qinghua, YAN Mingcai. Handbook of Elemental Abundance for Applied Geogechimistry[M]. Beijing:Geoligical Pulishing House, 2007.] [30] Taylor S R and McLenan S M. The Continental Crust:Its Composition and Evolution[M]. London:Blackwell Scientific Publications. 312.
[31] Dai S, Ren D, Chou C L, et al. Geochemistry of trace elements in Chinese coals:a review of abundances, genetic types, impacts on human health, and industrial utilization[J]. International Journal of Coal Geology, 2012, 94:3-21.
[32] Tian H Z, Wang Y, Xue Z G, et al. Trend and characteristics of atmospheric emissions of Hg, As, and Se from coal combustion in China, 1980-2007[J]. Atmospheric Chemistry and Physics, 2010, 10(23):11905-11919.
[33] 郑艳红,滕彦国. 中国大气中重金属钒的排放特征[J]. 环境科学与管理,2012,37(08):20-24. [ZHENG Yanhong, TENG Yanguo. E mission Characteristics of Vanadium in Air[J]. Environmental Science and Management, 2012, 37(08):20-24.]
[34] You C F, Xu X C. Coal combustion and its pollution control in China[J]. Energy, 2010, 35(11):4467-4472.
[35] 秦俊法. 中国燃油大气铅排放量估算[J]. 广东微量元素科学,2010,17(10):27-34. [QIN Junfa. Estim ation of Lead Emission to Atmospheric from Gasoline Com bustion[J]. Trace Element Science in Guangdong, 2010,17(10):27-34.]
[36] Li Q, Cheng H, Zhou T, et al. The estimated atmospheric lead emissions in China, 1990-2009[J]. Atmospheric Environment, 2012, 60:1-8.
[37] Streets D G, Hao J, Wu Y, et al. Anthropogenic mercury emissions in China[J]. Atmospheric Environment, 2005, 39(40):7789-7806.
[38] Nriagu J O, Pacyna J M. Quantitative assessment of worldwide contamination of air, water and soils by trace metals[J]. Nature, 1988, 333(6169):134-139.
[39] 郭广慧,陈同斌,宋波,等. 中国公路交通的重金属排放及其对土地污染的初步估算[J]. 地理研究,2007,26(05):922-930. [GUO Guanghui, CHEN Tongbin, SONG Bo, et al. Emissions of heavy metals from road traffic and effect of emitted lead on land contamination in China:A primary study[J]. Geographical Research, 2007, 26(05):922-930.]
[40] Councell T B, Duckenfield K U, Landa E R, et al. Tire-wear particles as a source of zinc to the environment[J]. Environmental Science & Technology, 2004, 38(15):4206-4214.
[41] 李波,林玉锁,张孝飞,等. 沪宁高速公路两侧土壤和小麦重金属污染状况[J]. 农村生态环境,2005,21(03):50-53 ,70.[LI Bo, LIN Yusuo, ZHANG Xiaofei, et al. H eavy metal pollution of the so ils and wheat grains alongside the Shanghai-Nanjing Expressway[J]. Rural Eco-Environment, 2005, 21(3):50-53, 70.]
[42] Gan H, Zhuo M, Li D, et al. Quality characterization and impact assessment of highway runoff in urban and rural area of Guangzhou, China[J]. Environmental Monitoring and Assessment, 2008, 140(1-3):147-159.
[43] 许海,邵婉晨,李光辉,等. 沪宁高速公路(常州段)两侧农田土壤重金属污染状况检测评价[J]. 江苏农业学报,2009,25(01):123-126. [XU Hai, SHAO Wanchen, LI Guanghui, et al. Assessment of Heavy Metal Pollution in Roadside Soils along Shanghai-Nanjing Highway(ChangzhouSection)[J].Jiangsu J.of Agr. Sci., 2009, 25(01):123-126.]
[44] 李波,林玉锁. 公路两侧农田土壤铅污染及对农产品质量安全的影响[J]. 环境监测管理与技术,2005,17(01):11-14. [LI Bo, LIN Yusuo. Assessment of Pb pollution in Roadside soils and its influence on quality security of Agricultural Product[J]. Management and Technology of Environmental Monitoring, 2005, 17(01):11-14.]
[45] Tian H, Gao J, Lu L, et al. Temporal trends and spatial variation characteristics of hazardous air pollutant emission inventory from municipal solid waste incineration in China[J]. Environmental Science & Technology, 2012, 46(18):10364-10371.
[46] 陈海滨,邓成,毛毅. 城镇生活垃圾资源化处理方案的技术经济比选研究[J]. 环境工程学报,2007,01(01):130-133. [CHEN Haibin, DENG Cheng, MAO Yi. Research on technical& economical comparison and optimization of municipal solid waste reclamation scheme[J]. Chinese Journal of Environmental Engineering, 2007,01(01):130-133.]
[47] Tian H, Cheng K, Wang Y, et al. Temporal and spatial variation characteristics of atmospheric emissions of Cd, Cr, and Pb from coal in China[J]. Atmospheric Environment, 2012, 50:157-163.
[48] Tian H Z, Wang Y, Xue Z G, et al. Trend and characteristics of atmospheric emissions of Hg, As, and Se from coal combustion in China, 1980-2007[J]. Atmospheric Chemistry and Physics, 2010, 10(23):11905-11919.
[49] Tian H Z, Lu L, Cheng K, et al. Anthropogenic atmospheric nickel emissions and its distribution characteristics in China[J]. Science of the Total Environment, 2012, 417:148-157.
[50] 邵学新,吴明,蒋科毅. 土壤重金属污染来源及其解析研究进展[J]. 广东微量元素科学,2007,14(04):1-6. [SHAO Xuexin, WU Ming, JIANG Keyi. Research Progress in Sources Identif ication of Soil HeavyMetal Pollution[J]. Trace Element Science in Guangdong, 2007, 14(4):1-6.]
[51] 李致春,桂和荣,孙林华. 河流沉积物中重金属来源分析方法研究进展[J]. 化学分析计量,2012,21(05):94-96. [LI Zhichun, GUI Herong, SUN Linhua. Research Progress on Source Analysis of Heavy Metal in River Sediments[J]. Chemical Analysis and Meterage, 2012,21(05):94-96.]
[52] Zhang W, Feng H, Chang J, et al. Lead (Pb) isotopes as a tracer of Pb origin in Yangtze River intertidal zone[J]. Chemical Geology, 2008, 257(3):257-263.
[53] Xu B, Yang X B, Gu Z Y,et al. The trend and extent of heavy metal accumulation over last one hundred years in the Liaodong Bay, China[J]. Chemosphere, 2009, 75:442-446.
[54] Liu J P, Xu K H, Li A C, et al. Flux and fate of Yangtze River sediment delivered to the East China Sea[J]. Geomorphology, 2007, 85(3):208-224.
[55] 顾家伟,王灿,Alaa Salem. 尼罗河三角洲与长江三角洲重金属污染对比研究[J]. 地球与环境,2013,41(03):233-241. [GU Jiawei, WANG Chan, Alaa Salem. The comparative study of Heavy Metal contamination between the Nile Delta and the Yangtze Delta[J].Earth and Environment, 2013,41(03):233-241.]
[56] Bird G. Provenancing anthropogenic Pb within the fluvial environment:Developments and challenges in the use of Pb isotopes[J]. Environment International, 2011, 37(4):802-819.
[57] Hao Y C, Guo Z G, Yang Z S, et al. Tracking historical lead pollution in the coastal area adjacent to the Yangtze River Estuary using lead isotopic compositions[J]. Environmental Pollution, 2008, 156:1325-1331.
[58] Kylander M E, Weiss D J, Martínez Cortizas A, et al. Refining the pre-industrial atmospheric Pb isotope evolution curve in Europe using an 8000 year old peat core from NW Spain[J]. Earth and Planetary Science Letters, 2005, 240(2):467-485.
[59] Lima A L, Bergquist B A, Boyle E A, et al. High-resolution historical records from Pettaquamscutt River basin sediments:Pb isotopes reveal a potential new stratigraphic marker[J]. Geochimica et cosmochimica acta, 2005, 69(7):1813-1824.
[60] Choi M S, Yi H I, Yang S Y, et al. Identification of Pb sources in Yellow Sea sediments using stable Pb isotope ratios[J]. Marine Chemistry, 2007, 107(2):255-274.
[61] 祁昌实,朱祥坤,戴民汉,等. 海洋沉积物的铁和锌同位素测定[J]. 地球化学,2012,41(03):197-206. [QI Changshi, ZHU Xiangkun, DAI Minhan, et al. High-precision measurements of Fe and Zn isotopic ratios in marine sediments[J]. Geochimica, 2012,41(03):197-206.]
[62] John S G, Genevieve Park J, Zhang Z, et al. The isotopic composition of some common forms of anthropogenic zinc[J]. Chemical Geology, 2007, 245(1):61-69.
[63] 梁莉莉,刘丛强,王中良,等. 铜锌同位素方法在环境地球化学研究中的应用[J]. 地球与环境,2006,34(01):81-89. [LIANG Lili, LIU Congqiang, WANG Zhongliang,et al. Environmental quality of heavy metals in surface sediments in the central region of the Bohai Sea[J]. Earth and Environment, 2006,34(01):81-89.]
[64] Bigalke M, Weyer S, Kobza J, et al. Stable Cu and Zn isotope ratios as tracers of sources and transport of Cu and Zn in contaminated soil[J]. Geochimica et Cosmochimica Acta, 2010, 74(23):6801-6813.
[65] Juillot F, Marechal C, Morin G, et al. Contrasting isotopic signatures between anthropogenic and geogenic Zn and evidence for post-depositional fractionation processes in smelter-impacted soils from Northern France[J]. Geochimica et Cosmochimica Acta, 2011, 75(9):2295-2308.
[66] Weiss D J, Rausch N, Mason T F D, et al. Atmospheric deposition and isotope biogeochemistry of zinc in ombrotrophic peat[J]. Geochimica et Cosmochimica Acta, 2007, 71(14):3498-3517.
[67] Thapalia A, Borrok D M, Van Metre P C, et al. Zn and Cu isotopes as tracers of anthropogenic contamination in a sediment core from an urban lake[J]. Environmental Science & Technology, 2010, 44(5):1544-1550.
[68] Duce R A, Liss P S, Merrill J T, et al. The atmospheric input of trace species to the world ocean[J].Global bicgechemical cycles, 1991,5(3):193-259.
[69] Viers J, Dupré B, Gaillardet J. Chemical composition of suspended sediments in World Rivers:new insights from a new database[J]. Science of the Total Environment, 2009, 407(2):853-868.
[70] McKee B A, Aller R C, Allison M A, et al. Transport and transformation of dissolved and particulate materials on continental margins influenced by major rivers:benthic boundary layer and seabed processes[J]. Continental Shelf Research, 2004, 24(7):899-926.
[71] Zhang J, Liu C L. Riverine composition and estuarine geochemistry of particulate metals in China-weathering features, anthropogenic impact and chemical fluxes[J]. Estuarine, Coastal and Shelf Science, 2002, 54(6):1051-1070.
[72] Zhang K and Gao H W. The characteristics of Asian-dust storms during 2000-2002:From the source to the sea[J]. Atmospheric Environment, 2007, 41(39):9136-9145.
[73] Mori I, Nishikawa M, Tanimura T, et al. Change in size distribution and chemical composition of kosa (Asian dust) aerosol during long-range transport[J]. Atmospheric Environment, 2003, 37(30):4253-4263.
[74] Yang Z S, Wang H J, Saito Y, et al. Dam impacts on the Changjiang (Yangtze) River sediment discharge to the sea:The past 55 years and after the Three Gorges Dam[J]. Water Resources Research, 2006, 42(4).
[75] 杨作升,李国刚,王厚杰,等. 55年来黄河下游逐日水沙过程变化及其对干流建库的响应[J]. 海洋地质与第四纪地质,2008,28(06):9-18. [YANG Zuosheng, LI Guogang, WANG Houjie, et al. Variation of daily water and sediment discharge in the Yellow River lower reaches in the past 55 years and its response to the dam operation on its main stream[J]. Marine Geology and Quaternary Geology, 2012, 28(06):279-290.]
[76] Yuan H, Song J, Li X, et al. Distribution and contamination of heavy metals in surface sediments of the South Yellow Sea[J]. Marine pollution bulletin, 2012, 64(10):2151-2159.
[77] 王长友,王修林,李克强,等. 东海陆扰海域铜、铅、锌、镉重金属排海通量及海洋环境容量估算[J].海洋学报,2010,32(04):62-76. [WANG Changyo, WANG Xiulin, LI Keqiang, et al. The estimation of copper, lead, zinc and cadminum fluxes into the sea area of the East China Sea interferenced by terrigenous matter and their environmental capacities[J]. Acta Oceanologica Sinica, 2010, 32(04):62-76.]
[78] 中国环保部.中国环境质量公告.2012.[Ministry of environmental protection of the People's Republic of China. Annural report of the national environment. 2012.] [79] Huang P, Li T, Li A, et al. Distribution, enrichment and sources of heavy metals in surface sediments of the North Yellow Sea[J]. Continental Shelf Research, 2014, 73:1-13.
[80] Hu L, Zhang G, Zheng B, et al. Occurrence and distribution of organochlorine pesticides (OCPs) in surface sediments of the Bohai Sea, China[J]. Chemosphere, 2009, 77(5):663-672.
[81] 中华人民共和国国家海洋局.国家海洋污染公告.2005.[NBO, Ministry of Environmental protection National Bureau of Oceanography of China. Bulletin of Marine Environmental Quality. 2005.] [82] Gao X, Chen C T A. Heavy metal pollution status in surface sediments of the coastal Bohai Bay[J]. Water Research, 2012, 46(6):1901-1911.
[83] 胡宁静,石学法,黄朋,等. 渤海辽东湾表层沉积物中金属元素分布特征[J]. 中国环境科学,2010,30(03):380-388. [HU Ningjing, SHI Xuefa, HUANG Peng, et al. Distribution of metals in surface sediments of Liaodong Bay, Bohai Sea[J]. China Environmental Science, 2010,30(3):380-388.]
[84] 秦延文,苏一兵,郑丙辉,等. 渤海湾表层沉积物重金属与污染评价[J]. 海洋科学,2007,31(12):28-33. [QIN Yanwen, SU Yibing, ZHENG Binghui, et al. Environmental quality of heavy metals in surface sediments in the central region of the Bohai Sea[J]. Marine Sciences 2007,31(12):28-33.]
[85] 罗先香,张蕊,杨建强,等. 莱州湾表层沉积物重金属分布特征及污染评价[J]. 生态环境学报,2010,19(02):262-269. [LUO Xianxiang, ZHANG Rui, YANG Jianqiang, et al. Distribution and pollution assessment of heavy metals in surface sediment in Laizhou Bay[J]. Ecology and Environmental Sciences, 2010, 19(02):262-269.]
[86] 胡宁静,石学法,刘季花,等. 莱州湾表层沉积物中重金属分布特征和环境影响[J]. 海洋科学进展,2011,29(01):63-72. [HU Ningjing, SHI Xuefa, LIU Jihua, et al. Distributions and Impacts of Heavy Metals in the Surface Sediments of the Laizhou Bay[J]. Advances in Marine Science, 2011, 29(01):63-72.]
[87] 张现荣,张勇,叶青,等. 辽东湾北部海域沉积物重金属环境质量和污染演化[J]. 海洋地质与第四纪地质,2012,32(02):21-29. [ZHANG Xianrong, ZHANG Yong, YE Qing, et al. Environment quality of Liaodong Bay and pollution evolution of heavy metals[J]. Marine Geology and Quaternary Geology, 2012,32(02):279-290.]
[88] Li X, Liu L, Wang Y, et al. Integrated assessment of heavy metal contamination in sediments from a coastal industrial basin, NE China[J]. PloS one, 2012, 7(6):e39690.
[89] 中华人民共和国国家海洋局.中国海洋环境质量公告. 2010.[NBO, Ministry of Environmental protection National Bureau of Oceanography of China. Bulletin of Marine Environmental Quality. 2010] [90] Gao X, Li P. Concentration and fractionation of trace metals in surface sediments of intertidal Bohai Bay, China[J]. Marine Pollution Bulletin, 2012, 64(8):1529-1536.
[91] 徐亚岩,宋金明,李学刚,等. 渤海湾表层沉积物各形态重金属的分布特征与生态风险评价[J]. 环境科学,2012,33(03):732-740. [XU Yayan, SONG Xueming, LI Xuegang, et al. Variation Characteristics and Potential Ecological Risk Assessment of Heavy Metals in the Surface Sediments of Bohai Bay[J]. Environmental Science, 2012, 33(03):732-740.]
[92] Gao X, Chen C T A. Heavy metal pollution status in surface sediments of the coastal Bohai Bay[J]. Water Research, 2012, 46(6):1901-1911.
[93] 李淑媛,郝静. 渤海湾及其附近海域沉积物中Cu,Pb,Zn,Cd环境背景值的研究[J]. 海洋与湖沼,1992,23(01):39-48. [LI Shuyan, HAO Jing. The study of environment background concentrations of Cu, Pb, Zn and Cd in the sediment of the Bohai Bay and its adjacent sea area[J]. Ocanologia et Limnologia Sinica, 1992, 23(01):39-48.]
[94] Yang S, Youn J S. Geochemical compositions and provenance discrimination of the central south Yellow Sea sediments[J]. Marine Geology, 2007, 243(1):229-241.
[95] 李淑媛,苗丰民,刘国贤. 北黄海沉积物中重金属分布及环境背景值[J]. 黄渤海海洋,1994,12(03):20-24. [LI Shuyuan, MIAO Fengmin, LIU Guoxian. The Distribution and Environmental Background Values of the Heavy Metals in the sediment of the North Huanghai Sea[J]. Journal of Oceanography of Huanghai&Bohai Sea, 1994,12(03):20-24.]
[96] 杜俊涛,陈洪涛,田琳. 北黄海表层沉积物中重金属含量及其污染评价[J]. 中国海洋大学学报(自然科学版),2010,40(Sup.):167-172.[DU Juntao, CHEN Hongtao, TIAN Lin. Heavy Metals in the Surface Sediments of the North Yellow Sea and Its Ecological Risk[J]. Preriodical of Ocean Univers ity of China, 2010(Natural Science), 40(Sup.):167-172.] [97] 张珂,王朝晖,冯杰,等. 芝罘湾表层沉积物中重金属的分布特征及潜在生态危害评价[J]. 分析测试学报,2011,30(06):593-599. [ZHANG Ke, WANG Chaohui, FENG Jie, et al. Distribution and Potential Ecological Risk Assessment of Heavy Metals in Surface Sediments from Zhifu Bay, the Yellow Sea[J]. Journal of Instrumental Analysis, 2011,30(06):593-599.]
[98] Sun Q, Liu D, Liu T, et al. Temporal and spatial distribution of trace metals in sediments from the northern Yellow Sea coast, China:implications for regional anthropogenic processes[J]. Environmental Earth Sciences, 2012, 66(3):697-705.
[99] Dai J, Song J, Li X, et al. Environmental changes reflected by sedimentary geochemistry in recent hundred years of Jiaozhou Bay, North China[J]. Environmental Pollution, 2007, 145(3):656-667.
[100] Deng B, Zhang J, Zhang G, et al. Enhanced anthropogenic heavy metal dispersal from tidal disturbance in the Jiaozhou Bay, North China[J]. Environmental Monitoring and Assessment, 2010, 161(1-4):349-358.
[101] Guo Z, Lin T, Zhang G, et al. High-resolution depositional records of polycyclic aromatic hydrocarbons in the central continental shelf mud of the East China Sea[J]. Environmental Science & Technology, 2006, 40(17):5304-5311.
[102] 何书锋,李广雪,史经昊. 胶州湾表层沉积物重金属元素分布特征及其影响因素[J]. 海洋地质前沿,2013,29(04):41-48. [HE Shufeng, LI Guangxue,SHI Jinghao. Distribtution of heavy metals in suficial sediments of Jiaozhou Bay and its influencing factors[J]. Marine Geology Frontiers.2013,29(04):41-48.]
[103] Duan L, Song J, Yuan H, et al. Spatio-temporal distribution and environmental risk of arsenic in sediments of the East China Sea[J]. Chemical Geology, 2013, 340:21-31.
[104] Deng B, Zhang J, Wu. Y. Recent sediment accumulation and carbon burial in the East China Sea. Global Biogeochemial Cycles[J].200620(3):466-480.
[105] Lin S, Hsieh I J, Huang K M, et al. Influence of the Yangtze River and grain size on the spatial variations of heavy metals and organic carbon in the East China Sea continental shelf sediments[J]. Chemical Geology, 2002, 182(2):377-394.
[106] 中华人民共和国海洋局.中国海洋环境质量公告[R].2008.[NBO, Ministry of Environmental protection National Bureau of Oceanography of China. Bulletin of Marine Environmental Quality[R]. 2008] [107] 赵宝刚,邵秘华,鲍永恩,等. 东海表层沉积物中重金属集散特征及变化规律[J]. 大连海事大学学报,2008,34(03):13-16 ,20.[ZHAO Baogang, SHAO Mihua, PAO Yongen, et al. The features of concentration and dispersion of the heavy metals and their changing patterns in surface sediment of East China Sea[J]. Journal of Dalian Maritime University, 2008, 34(03):02:13-16, 20.]
[108] 栗俊,鲍永恩,刘广远,等. 东海陆架沉积物中重金属地球化学研究[J]. 海洋环境科学,2007,26(01):63-66. [LI Jun, PAO Yongen, LIU Guangyuan, et al. Study on geochemistry of heavy metals in the sediment in the East China Sea continental shelf[J]. Marine Environmental Science, 2007, 26(01):63-66.]
[109] Liu S, Shi X, Liu Y, et al. Concentration distribution and assessment of heavy metals in sediments of mud area from inner continental shelf of the East China Sea[J]. Environmental Earth Sciences, 2011, 64(2):567-579.
[110] 董爱国,翟世奎,ZABEL Matthias,等. 长江口及邻近海域表层沉积物中重金属元素含量分布及其影响因素[J]. 海洋学报,2009,31(06):54-68. [DONG Aiguo, ZHAI Shikui, ZABEL Matthias, et al. The distribution of heavy metal contents in surface sediments of the Changjiang Estuary in China and surrounding coastal areas[J]. Acta Oceanologica Sinica, 2009,31(06):54-68.]
[111] 张弛,高效江,宋祖光,等. 杭州湾河口地区表层沉积物中重金属的分布特征及污染评价[J]. 复旦大学学报:自然科学版,2008,47(04):535-540. [ZHANG Chi, GAO Xiaojiang, SONG Zhuguang, et al. Heavy Metal Distribution and Pollution Assessmentin the Surface Sediments of Hangzhou Bay[J]. Journal of Fudan University (Natural Science), 2008,47(04):535-540.]
[112] Yu R, Yuan X, Zhao Y, et al. Heavy metal pollution in intertidal sediments from Quanzhou Bay, China[J]. Journal of Environmental Sciences, 2008, 20(6):664-669.
-
期刊类型引用(8)
1. 裴宇，张生银，房嬛，陈永欣，张顺存，邵明，雷天柱. 陆架边缘海环境下金属元素与有机质富集关系探讨——以南黄海表层沉积物为例. 沉积学报. 2022(01): 136-148 . 
百度学术
2. 汤世凯，张杰，于晓静，陶志斌，李金鹏. 山东丁字湾海域沉积物重金属含量、分布及与粒径之间的关系研究. 现代地质. 2020(05): 928-935 . 百度学术
3. 史戈，曾辉，常文静. 我国海岸带污染生态环境效应研究现状. 生态学杂志. 2019(02): 576-585 . 百度学术
4. 何中发，杨守业，赵宝成，李晓，谢建磊，温晓华. 长江口地区近1500年以来沉积物重金属含量变化及其对流域环境响应. 海洋地质与第四纪地质. 2019(02): 21-30 . 本站查看
5. 石一茜，赵旭，俞锦辰，林军，韩星雨，刘臻，黄宏. 马鞍列岛人工鱼礁修复海域沉积物重金属形态组成及垂直分布特征. 水产学报. 2019(09): 1952-1962 . 百度学术
6. 梁胜跃，刘建东，郭炳跃，徐明钻，祁超，金志鹏. 江苏省连云港市前三岛附近海域地球化学特征及风险指标探讨. 物探与化探. 2017(05): 963-971+990 . 百度学术
7. 周嘉源，刘珊珊，张晓波. 山东半岛南部海域沉积物中重金属元素研究现状. 海洋地质前沿. 2016(06): 39-42+49 . 百度学术
8. 李玉，李宏观. 连云港近海沉积物重金属历史分布特征及其来源. 水生态学杂志. 2016(06): 59-67 . 百度学术
其他类型引用(6)
计量
- 文章访问数: 2215
- HTML全文浏览量: 250
- PDF下载量: 21
- 被引次数: 14
下载:
