浙闽河流碎屑锆石U-Pb年龄分布特征及其影响因素

Characteristics of detrital zircon U-Pb age distribution and influencing factors in the rivers of Zhejiang and Fujian Provinces, China

  • 摘要: 河流碎屑锆石U-Pb年龄组成能够综合反映锆石源区所经历的构造、岩浆与变质活动,是指示沉积物物源以及从源到汇过程的理想示踪剂。然而,一些基于现代河流碎屑锆石的研究认为,锆石年龄谱信号受到沉积物搬运、分选、混合过程的影响,并不能真实反映物源。本文以浙闽流域7条代表性河流为研究对象,通过激光剥蚀-电感耦合等离子体质谱技术揭示其碎屑锆石U-Pb年龄的分布特征,并结合全样粒度、碎屑锆石粒度与形态学分析,探究水动力分选对流域锆石年龄谱可能产生的影响。研究表明,浙闽河流碎屑锆石U-Pb年龄分布具有显著的空间差异性。钱塘江碎屑锆石U-Pb年龄以80~180 Ma、190~524 Ma、677~916 Ma三个主要区间为特征;椒江具有一个125 Ma左右燕山期的年龄峰;瓯江碎屑锆石以113~190 Ma和1707~1897 Ma两个年龄区间为特征;闽江碎屑锆石存在76~244 Ma、374~457 Ma、732~816 Ma、16221935 Ma四个主要年龄区间;木兰溪以100 Ma的白垩纪峰与142 Ma的侏罗纪峰为特征;晋江流域碎屑锆石年龄集中在78~175 Ma;九龙江存在75~120 Ma、120~180 Ma和192~313 Ma三个年龄区间。其中,燕山期120~180 Ma侏罗纪—白垩纪年龄区间在所有流域中均有发现。结合流域构造、火山岩与沉积地层信息,本文认为研究区碎屑锆石年龄的空间分布特征与中生代以来太平洋板块向欧亚板块俯冲引发的中国东部大规模构造、岩浆活动相关。此外,锆石等效球径与形态学研究发现研究区河流的锆石粒度大小与年龄无显著相关性,指示了是物源而非水动力分选对锆石年龄谱有显著影响。然而,锆石磨圆度与锆石年龄呈现出锆石年龄越老,磨圆度越高的趋势,表明长期搬运和沉积旋回过程对锆石年龄谱的解译存在潜在影响。

     

    Abstract: U-Pb age compositions of fluvial detrital zircon comprehensively reflect tectonic, magmatic, and metamorphic activities of zircon sources. It serves as a reliable tracer for provenance analysis and source-to-sink processes, and has become popular in revealing river evolution and quantifying the relative contribution of sediments. However, a few studies on modern fluvial detrital zircon have raised concerns that zircon age distributions are affected by sediment transport, sorting, and mixing processes. Therefore, it is crucial to examine the controlling and influencing factors of zircon age distributions in fluvial source-sink systems. We studied the U-Pb ages of detrital zircon in seven catchments in Zhejiang and Fujian provinces, from which the distribution characteristics of detrital zircon U-Pb ages were determined using laser ablation-inductively coupled plasma (LA-ICP-MS) technology. Through bulk samples and zircon grain-size analyses, the potential influence of hydrodynamic sorting on the age spectrum of the basins was revealed. Results show significant spatial differences in the U-Pb age distributions of detrital zircon in the rivers in Zhejiang and Fujian Provinces. The detrital zircon U-Pb ages of the Qiantang River are characterized by three main age groups: 80~180 Ma, 190~524 Ma, and 677~916 Ma. The Jiaojiang River has only one age peak of the Yanshanian period at approximately 125 Ma. There are two characteristic age groups, 113~190 Ma and 1707~1897 Ma, in the detrital zircon of the Oujiang River. The detrital zircon of the Minjiang River has four main age intervals: 76~244 Ma, 374~457 Ma, 732~816 Ma, and 1622~1935 Ma. The main zircon age peaks of the Mulanxi River detrital zircon are the Cretaceous peak, ca. 100 Ma, and the Jurassic peak, ca. 142 Ma. The ages of detrital zircons in the Jinjiang River Basin are all concentrated between 78 and 175 Ma. The detrital zircons in the Jiulong River have three age groups: 75~120 Ma, 120~180 Ma, and 192~313 Ma. Nevertheless, the age spectra of detrital zircons in the seven rivers all contain groups from the Jurassic-Cretaceous of the Yanshanian period, ranging from 120 to 180 Ma. The spatial distribution characteristics of detrital zircon age in the Zhejiang-Fujian provinces are associated with the large-scale magmatic activities in East China, which were caused by the subduction of the Pacific Plate beneath the Eurasian Plate since the Mesozoic. More interestingly, zircon morphology analysis revealed no significant correlation between the zircon grain size of the seven rivers and their U-Pb ages, indicating that provenance, rather than hydrodynamic sorting, had a significant impact on the zircon age spectrum. However, study on zircon equivalent sphere diameter and morphology showed a trend that the older the zircon, the higher the roundness, which suggests that the distribution of zircon grain shapes is influenced by the long-term transportation and sedimentary cycling processes.

     

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